Impacts of Mesoscale Cloud Organization on Aerosol-Induced Cloud Water Adjustment and Cloud Brightness

The role of mesoscale cellular convection (MCC) in regulating aerosol-induced cloud brightness remains unaddressed. Using 7 years of satellite-based observations of cloud water adjustment to aerosol-induced perturbations for closed MCCs across different sizes (8, 16, 32, and 64 km) over the North Atlantic Ocean, we show that MCC cell-size plays a nontrivial role in regulating aerosol-induced cloud brightness via cloud water adjustment. In cells that are primarily non-precipitating, the adjustment in small-scale MCCs can be 10 times more negative than in large-scale MCCs, consistent with stronger evaporation via cloud top entrainment. Consequently, the response of cloud brightness is significantly stronger for large-scale MCCs. We also find notable intra-cell co-variability between cloud liquid water path (LWP) and drop concentration (N_d) within MCCs that varies with cell size. Erroneously considering such co-variability as a LWP response to N_d can lead to a significant positive bias, especially for small scale MCCs.. Authors: Zhou, Xiaoli [National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States); Univ. of Colorado, Boulder, CO (United States)] (ORCID:0000000231342092); Feingold, Graham [National Oceanic and Atmospheric Administration (NOAA), Boulder, CO (United States)] (ORCID:0000000207742926). DOE Contract: 89243020SSC000055. Subjects: 54 ENVIRONMENTAL SCIENCES