GOTHIC Aerosol Source Depletion Studies

Pacific Northwest National Laboratory has continued work to develop an aerosol-laden flow modeling capability with the Generation of Thermal Hydraulic Information in Containment (GOTHIC^TM) computer code to perform simulations for thermal hydraulic conditions and aerosol transport and deposition in spent fuel casks. This report describes our recent work to expand our model that was originally developed in 2019 to allow for thermal characterization, carrier gas flow determination, and tracking of particulate behavior throughout the entire canister volume. This was achieved through conversion of decay heat source in all fuel tubes within the model from heaters to thermal conductors in GOTHIC as well as remeshing the internal volume of the canister. These model improvements allowed for simulations of base case scenarios for comparison of similar efforts by our collaborators with alternative tools at Sandia and Oak Ridge. Several characteristics of the GOTHIC code were elucidated by this effort and were documented for consideration in how the code is used for this effort moving forward. For instance, treatment of particle size distributions, initial spatial distributions, mesh gradients, and minimum volume concentrations were identified as important issues for consideration. Ultimately, the current version of the code is capable of tracking temperatures, flow rates, and particle behavior throughout the canister internal volume. This report presents predicted depletion times and preferred deposition patterns within the canister. Additionally, this report documents code performance and insights for further model development and use for comparisons to other codes and for predicting system behavior in experiments being performed and planned by our collaborators.. Authors: Lanza, Mark S. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)]; Leimon, Michael [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)]; Elsawi, Mohamed A. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)]; Casella, Andrew M. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)] (ORCID:0000000240536593). DOE Contract: AC05-76RL01830. Subjects: Aerosol; Dry Cask Storage System; GOTHIC; spend nuclear fuel; Thermal Hydraulic Analysis