Incorporating geological structure into sensitivity analysis of subsurface contaminant transport

Simulating subsurface contaminant transport at the kilometer-scale often entails modeling reactive flow and transport within and through complex geologic structures. These structures are typically meshed by hand and as a result geologic structure is usually represented by one or a few deterministically generated geological models for uncertainty studies of flow and transport in the subsurface. Uncertainty in geologic structure can have a significant impact on contaminant transport. In this study, the impact of geologic structure on contaminant tracer transport in a shale formation is investigated for a simplified generic deep geologic repository for permanent disposal of spent nuclear fuel. An open-source modeling framework is used to perform a sensitivity analysis study on transport of two tracers from a generic spent nuclear fuel repository with uncertain location of the interfaces between the stratum of the geologic structure. The automated workflow uses sampled realizations of the geological structural model in addition to uncertain flow parameters in a nested sensitivity analysis. Concentration of the tracers at observation points within, in line with, and downstream of the repository are used as the quantities of interest for determining model sensitivity to input parameters and geological realization. Finally, the results of the study indicate that the location of strata interfaces in the geological structure has a first-order impact on tracer transport in the example shale formation, and that this impact may be greater than that of the uncertain flow parameters.. Authors: Bigler, Lisa Amelia [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)] (ORCID:0000000337858660); LaForce, Tara Catherine [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)]; Swiler, Laura Painton [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)]. DOE Contract: NA0003525. Subjects: 12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES; 58 GEOSCIENCES; Automated mesh generation; Deep geologic disposal; Geological structure uncertainty; Spent nuclear fuel; Voronoi mesh